Prospective Inventory of Radioactive Materials and Waste Management Study in French Nuclear Fleet

 
AIEA Conference – Vienna – 
June, 26
th
 2019
 
 
 
C. Chabert 
, E. Touron, A. Saturnin, F. Courtin, G. Krivtchik, Ph. Miranda, G. Martin, JL. Girotto
with the collaboration of French industrial partners EDF, ORANO, FRAMATOME
 
Atomic Energy and Alternative Energies Commission - 
www.cea.fr
 
Prospective inventory of radioactive materials
and waste produced by the French nuclear
fleet according to different plutonium multiple
recycling options in the frame of the French
law for waste management
 
C
O
N
T
E
X
T
 
2
 
 
In accordance with the French Act of 28 June 2006 on the
sustainable management of radioactive materials and waste, the
CEA in partnership with EDF, Orano and Framatome, has studied
prospective scenarios using different fuel cycle options:
o
 
 Open cycle,
o
 
Mono-recycling
 of plutonium and uranium in 
PWRs
 (current
option for the French nuclear power fleet),
o
 
Multiple recycling 
of reusable materials in 
SFRs
o
 
Multiple recycling 
of plutonium in 
PWRs
 
The results of this study has been submitted by the CEA to the
Ministry of Energy within the scope of Article 51 of the Ministerial
Order dated 23 February on the French National Radioactive
Materials and Waste Management Plan (PNGMDR).
 
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3
 
Progressive implementation of SFRs through successive phases:
Each phase envolves the more significant deployment of fast
reactors with its own growth objective
 
Phase 0: hypothetical French fleet having in an open cycle configuration only
 
4
 
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However, SFRs may not become economically competitive in the next few
decades as uranium resources would remain readily available
Advanced fuel technologies, called CORAIL-2000 and MIX, are applied to enable
multiple recycling of plutonium in standard PWRs
The main objectives of these scenarios consist in stabilizing the plutonium
inventory as well as all spent fuel stockpiles
 
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Few assumptions
o
The nuclear energy production remains steady at its current level, about 420TWhe/y
o
The starting point is the actual situation (with 58 PWR)
o
A lifespan of 60 years for future reactors (PWR and FR)
o
A lifespan of 50 years for the fuel cycle plants (La Hague/Melox facilities renewal near 2040)
o
For the FR fleet, the CFV core concept (low sodium void effect) (CEA) is considered
   
(600MWe, 1GWe and 1,45GWe)
 
For scenarios involving the progressive deployment of SFRs:
o
    Start-up of commercial SFRs: 25 years after the industrial commissioning of the demonstrator
 
      (assumed in this study to be in 2039), i.e. in the mid-2060s
o
    This timescale takes into account the need for sufficient feedback from the operation of
 
       the demonstrator and for realistic lead times for technical and regulatory actions
 
For scenarios involving the multiple recycling of Pu in PWRs:
o
   The industrial deployment of CORAIL and MIX concepts would be theoretically possible
 
      in 2045
o
    A timescale that seems at this stage in the studies to be reasonable, allowing qualification
 
      of these new fuel products.
 
 
 
 
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The transition from phase A to phase D improves - at each phase - the
quantities which are characteristic of the sustainable management of materials
Each phase makes its possible to improve the industrial maturity of the fast
reactors whose integration into phase B remains very minor (4,5% of the fleet)
 
8
 
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Multi-recycling of Pu in PWRs can lead to additional savings in uranium
     resources up to about 10% compared with the current once-through recycling
     in a configuration where reprocessed uranium is recycled
    (for a total exceeding 25% compared with an open fuel cycle)
MIX/ CORAIL concepts enable to recycle all spent fuel and stabilize Pu inventory
 
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9
 
o
Scenario ABCD1 involves the successive deployment of all phases,
 
starting with phase A (once-through recycling of Pu in PWRs), then
 
phase B (stabilisation of spent PWR MOX by recycling in a few SFRs),
 
followed by phase C (stabilisation of the Pu inventory using a symbiotic
 
PWR-SFR fleet), and finally phase D1 (100% SFR fleet)
o
Scenario ABCD2 ends with a hybrid fleet comprising SFRs and 100% MOX PWRs
o
Scenario ABD2 : an alternative to scenario ABCD2 where deployment of D2 is accelerated
 
(this scenario could apply in the case where the price of natural uranium rises rapidly or
 
there is a shortage of natural uranium).
 
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Open cycle
Once-recycling
ABCD1
ABCD2
ABD2
 
Open cycle
 
Open cycle
 
Open cycle
 
Once-recycling
 
Once-recycling
 
Once-recycling
 
Multi-recycling
 
Multi-recycling
 
Multi-recycling
 
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11
 
Scenarios implementing MIX/CORAIL concepts
 
Example: concept MIX 9,54% Pu associated with ERU EPR
 
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Self-sufficiency with respect to natural uranium can only be achieved by
opting for the closed fuel cycle, i.e. deployment of SFRs
Compared with scenario A, the consumption of natural uranium in the
MIX/CORAIL scenarios without ERU management is always higher by about
10 to 15% depending on the Pu content
In a configuration where reprocessed U is recycled, the multiple recycling of
Pu in PWRs can lead to additional savings in U resources
 
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But the Pu multi-recycling in PWRs increases the production of minor actinides
 up to 4.2 - 4.5 t/year  (vs. 3.3 t/year for “step A": increase ~ 30%)
 
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14
 
The waste disposal surface area required for the different options has been assessed in terms
       of the thermo-hydro mechanical (THM) and thermal design criteria
        relying on data provided by Andra, corresponding to current hypothesis of CIGEO project
This study does not pre-empt the location of the disposal site for the waste considered,
       nor any evolution or optimisations of the disposal design
For this study: clayey rock similar to the layer of argillaceous rock studied in the
        Meuse/ Haute-Marne region for the Cigéo project
 
Surface area required for HLW for a period of 60 years
 and after an interim storage periode of 80 years
 
A large quantity of spent fuel emitting high thermal
releases in phases 0, A and B will also require disposal
and thus a large disposal surface area
 
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C
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15
 
CEA in collaboration with EDF, Framatome and Orano has studied the industrial
feasibility of scenarios involving the 
progressive deployment of multiple recycling
of Pu in French sodium fast reactors and also in PWRs
A deployment of 
about 4,5% of SFR (~3 GWe) in the French fleet 
would be
sufficient 
to stabilise the interim storage of spent PWR MOX fuel 
(Phase B)
It is possible to 
stabilise the Pu inventory 
by deploying a symbiotic PWR-SFR fleet
with 
about 30% of SFR in the fleet
 (Phase C)
A full deployment of SFR or a mixed fleet comprising 75% breeder FRs and 25%
PWR fuelled with 100% MOX allows our 
independance on natural uranium
resources 
(Phase D)
This independance could be reached about 60 years earlier with a faster
deployment of SFR
 
( Scenario ABD compared ABCD)
 
 
 
M
A
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C
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L
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16
 
Recycling of Pu with MIX and CORAIL fuel assemblies in PWRs by the middle
of the century could lead to a stabilization of spent fuel and plutonium inventories
 
Small savings on U resource consumption may be reached only when considering
 the recycling of reprocessed U into ERU fuels
 
Industrial feasibility is under evaluation
(
requires adaptations of the fuel cycle plants or even new facilities according
to design and fuel capacity manufacturing and treatment)
 
Waste disposal footprint
:
 - 
only the disposal surface area required for vitrified waste packages has
   been estimated, considering current hypothesis of the French disposal project
-
These studies are still ongoing in collaboration with Andra to estimate the
   surface area required to dispose of the non-recycled spent fuels
 
 
 
 
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The study conducted by the French Atomic Energy Commission in collaboration with industrial partners like EDF, Orano, and Framatome explores different plutonium recycling options in the French nuclear fleet. It assesses scenarios involving open cycle, mono-recycling, and multiple recycling of plutonium and uranium in various reactor types. The study aims to comply with the French law on radioactive waste management and has implications for the sustainable future of nuclear energy in France. Advanced fuel technologies are also considered to stabilize plutonium inventories and spent fuel stockpiles. The transition to fast reactors is discussed, highlighting the challenges and objectives of each phase.

  • Radioactive Materials
  • Waste Management
  • French Nuclear Fleet
  • Plutonium Recycling
  • Nuclear Energy

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  1. Prospective inventory of radioactive materials and waste produced by the French nuclear fleet according to different plutonium multiple recycling options in the frame of the French law for waste management AIEA Conference Vienna June, 26th 2019 C. Chabert , E. Touron, A. Saturnin, F. Courtin, G. Krivtchik, Ph. Miranda, G. Martin, JL. Girotto with the collaboration of French industrial partners EDF, ORANO, FRAMATOME Atomic Energy and Alternative Energies Commission - www.cea.fr June, 26th2019 Commissariat l nergie atomique et aux nergies alternatives

  2. CONTEXT In accordance with the French Act of 28 June 2006 on the sustainable management of radioactive materials and waste, the CEA in partnership with EDF, Orano and Framatome, has studied prospective scenarios using different fuel cycle options: o Open cycle, o Mono-recycling of plutonium and uranium in PWRs (current option for the French nuclear power fleet), o Multiple recycling of reusable materials in SFRs o Multiple recycling of plutonium in PWRs The results of this study has been submitted by the CEA to the Ministry of Energy within the scope of Article 51 of the Ministerial Order dated 23 February on the French National Radioactive Materials and Waste Management Plan (PNGMDR). June, 26th2019 2 Commissariat l nergie atomique et aux nergies alternatives

  3. FUEL CYCLE TRANSITION SCENARIOS Progressive implementation of SFRs through successive phases: Each phase envolves the more significant deployment of fast reactors with its own growth objective Phase 0: hypothetical French fleet having in an open cycle configuration only June, 26th2019 3 Commissariat l nergie atomique et aux nergies alternatives

  4. FUEL CYCLE TRANSITION SCENARIOS However, SFRs may not become economically competitive in the next few decades as uranium resources would remain readily available Advanced fuel technologies, called CORAIL-2000 and MIX, are applied to enable multiple recycling of plutonium in standard PWRs The main objectives of these scenarios consist in stabilizing the plutonium inventory as well as all spent fuel stockpiles June, 26th2019 4 Commissariat l nergie atomique et aux nergies alternatives

  5. MULTI-RECYCLING CONCEPTS IN PWRS CORAIL and MIX concepts studied in CEA near 2000 MIX assembly - Homogeneous concept - 1 type of rods within assemblies - MOX rods with a support of enriched uranium to compensate for the degradation of the Pu isotopy - Constant Pu content, 3 cases in our study (8%, 9,54%,12%) - Pu consumption -43kg/TWhe (MIX 9,54%) CORAIL assembly design with 84 MOX rods - Heterogeneous concept - 2 types of rods within assemblies: UOX and MOX - U235 fixed (~5%) and Pu ajusted to compensate the Pu isotopic degradation (<12%) - Pu consumption 0kg/TWhe June, 26th2019 5 Commissariat l nergie atomique et aux nergies alternatives

  6. ASSUMPTIONS Few assumptions o The nuclear energy production remains steady at its current level, about 420TWhe/y o The starting point is the actual situation (with 58 PWR) o A lifespan of 60 years for future reactors (PWR and FR) o A lifespan of 50 years for the fuel cycle plants (La Hague/Melox facilities renewal near 2040) o For the FR fleet, the CFV core concept (low sodium void effect) (CEA) is considered (600MWe, 1GWe and 1,45GWe) For scenarios involving the progressive deployment of SFRs: o Start-up of commercial SFRs: 25 years after the industrial commissioning of the demonstrator (assumed in this study to be in 2039), i.e. in the mid-2060s o This timescale takes into account the need for sufficient feedback from the operation of the demonstrator and for realistic lead times for technical and regulatory actions For scenarios involving the multiple recycling of Pu in PWRs: o The industrial deployment of CORAILand MIX concepts would be theoretically possible in 2045 o Atimescale that seems at this stage in the studies to be reasonable, allowing qualification of these new fuel products. June, 26th2019 6 Commissariat l nergie atomique et aux nergies alternatives

  7. FR DEPLOYMENT MAIN CHARACTERISTICS FOR EACH PHASES A B C D2 D1 Open cycle (0) 0 Fraction of SFRs in the fleet Unat consumption (t/year) Pu inventory 0% 4.5% 31% 73% 100% 6000 5700 3400 0 0 7500 7.2 6.8 Stabilised Stabilised Stabilised 9.9 (t/year) Minor actinide inventory (t/year) Increase in the spent fuel inventory (t/y) 3.3 3.1 4.4 3.4 2.3 2.7 180 130 0 0 0 950 The transition from phase A to phase D improves - at each phase - the quantities which are characteristic of the sustainable management of materials Each phase makes its possible to improve the industrial maturity of the fast reactors whose integration into phase B remains very minor (4,5% of the fleet) June, 26th2019 7 Commissariat l nergie atomique et aux nergies alternatives

  8. MULTIPLE RECYCLING OF PU IN PWRS MAIN CHARACTERISTICS FOR EACH PHASES Multi-recycling of Pu in PWRs can lead to additional savings in uranium resources up to about 10% compared with the current once-through recycling in a configuration where reprocessed uranium is recycled (for a total exceeding 25% compared with an open fuel cycle) MIX/ CORAIL concepts enable to recycle all spent fuel and stabilize Pu inventory June, 26th2019 8 Commissariat l nergie atomique et aux nergies alternatives

  9. FUEL CYCLE TRANSITION SCENARIOS SCENARIOS INVOLVING THE PROGRESSIVE DEPLOYMENT OF SFRS Scenario ABCD1 involves the successive deployment of all phases, starting with phase A (once-through recycling of Pu in PWRs), then phase B (stabilisation of spent PWR MOX by recycling in a few SFRs), followed by phase C (stabilisation of the Pu inventory using a symbiotic PWR-SFR fleet), and finally phase D1 (100% SFR fleet) o Scenario ABCD2 ends with a hybrid fleet comprising SFRs and 100% MOX PWRs o Scenario ABD2 : an alternative to scenario ABCD2 where deployment of D2 is accelerated (this scenario could apply in the case where the price of natural uranium rises rapidly or there is a shortage of natural uranium). o June, 26th2019 9 Commissariat l nergie atomique et aux nergies alternatives

  10. SCENARIOS INVOLVING THE PROGRESSIVE DEPLOYMENT OF SFRS - MAIN RESULTS 2000 Consommation d'uranium naturel (kt) 1800 2400 Open cycle Open cycle Once-recycling 2200 1600 2000 1400 Once-recycling Inventaire en plutonium (t) 1800 1200 1600 1000 1400 800 Multi-recycling 1200 600 Multi-recycling 1000 400 800 200 600 0 400 2015 2045 2075 2105 2135 2165 2195 200 2015 2045 2075 2105 2135 2165 2195 A ABCD1 ABCD2 ABD2 Cycle ouvert Cycle Ouvert (0) Pu inventory stabilized A ABCD1 ABCD2 ABD2 Unat consumption decreased until 0 80 Open cycle Inventaire de combustibles us s (kt) 70 Once-recycling Open cycle Once-recycling ABCD1 ABCD2 ABD2 60 A 50 ABCD1 40 ABCD2 Multi-recycling 30 ABD2 Cycle ouvert 20 10 0 2015 Phase C: spent fuel inventory stabilized 2045 2075 2105 2135 2165 2195 June, 26th2019 10 Commissariat l nergie atomique et aux nergies alternatives

  11. SCENARIOS INVOLVING THE MULTIPLE RECYCLING OF PU IN PWRS Scenarios implementing MIX/CORAIL concepts Example: concept MIX 9,54% Pu associated with ERU EPR June, 26th2019 11 Commissariat l nergie atomique et aux nergies alternatives

  12. NATURAL URANIUM CONSUMPTION 1800 Consommation d'uranium naturel (kt) 1600 1400 1200 1000 800 600 400 200 0 2015 2045 2075 2105 2135 2165 2195 A ABCD1 ABD2 MIX 9,54% MIX 9,54% avec URE CORAIL Self-sufficiency with respect to natural uranium can only be achieved by opting for the closed fuel cycle, i.e. deployment of SFRs Compared with scenario A, the consumption of natural uranium in the MIX/CORAIL scenarios without ERU management is always higher by about 10 to 15% depending on the Pu content In a configuration where reprocessed U is recycled, the multiple recycling of Pu in PWRs can lead to additional savings in U resources June, 26th2019 12 Commissariat l nergie atomique et aux nergies alternatives

  13. STABILIZATION OF SPENT FUELS AND OF THE PLUTONIUM INVENTORY Stabilization of the total SF quantity near 2060 Stabilization of the Pu inventory achieved from ~ 2060 in all presented scenarios But the Pu multi-recycling in PWRs increases the production of minor actinides up to 4.2 - 4.5 t/year (vs. 3.3 t/year for step A": increase ~ 30%) June, 26th2019 13 Commissariat l nergie atomique et aux nergies alternatives

  14. WASTE AND GEOLOGICAL DISPOSAL The waste disposal surface area required for the different options has been assessed in terms of the thermo-hydro mechanical (THM) and thermal design criteria relying on data provided by Andra, corresponding to current hypothesis of CIGEO project This study does not pre-empt the location of the disposal site for the waste considered, nor any evolution or optimisations of the disposal design For this study: clayey rock similar to the layer of argillaceous rock studied in the Meuse/ Haute-Marne region for the Cig o project Surface area required for HLW for a period of 60 years and after an interim storage periode of 80 years SPENT FUEL: Annual thermal power (kW/y) to be stored (after interim storage during 80 y) 600 500 400 300 200 100 0 A large quantity of spent fuel emitting high thermal releases in phases 0, A and B will also require disposal and thus a large disposal surface area June, 26th2019 14 Commissariat l nergie atomique et aux nergies alternatives

  15. MAIN CONCLUSIONS CEA in collaboration with EDF, Framatome and Orano has studied the industrial feasibility of scenarios involving the progressive deployment of multiple recycling of Pu in French sodium fast reactors and also in PWRs A deployment of about 4,5% of SFR (~3 GWe) in the French fleet would be sufficient to stabilise the interim storage of spent PWR MOX fuel (Phase B) It is possible to stabilise the Pu inventory by deploying a symbiotic PWR-SFR fleet with about 30% of SFR in the fleet (Phase C) A full deployment of SFR or a mixed fleet comprising 75% breeder FRs and 25% PWR fuelled with 100% MOX allows our independance on natural uranium resources (Phase D) This independance could be reached about 60 years earlier with a faster deployment of SFR ( Scenario ABD compared ABCD) June, 26th2019 15 Commissariat l nergie atomique et aux nergies alternatives

  16. MAIN CONCLUSIONS Recycling of Pu with MIX and CORAIL fuel assemblies in PWRs by the middle of the century could lead to a stabilization of spent fuel and plutonium inventories Small savings on U resource consumption may be reached only when considering the recycling of reprocessed U into ERU fuels Industrial feasibility is under evaluation (requires adaptations of the fuel cycle plants or even new facilities according to design and fuel capacity manufacturing and treatment) Waste disposal footprint: - only the disposal surface area required for vitrified waste packages has been estimated, considering current hypothesis of the French disposal project - These studies are still ongoing in collaboration with Andra to estimate the surface area required to dispose of the non-recycled spent fuels June, 26th2019 16 Commissariat l nergie atomique et aux nergies alternatives

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