Nuclear Decays and Reactions in Stellar Astrophysics

When Michel’s favorite tiny electrons
fool the big atomic nuclei in the skies
Stellar Nucleosynthesis  and Cosmochronology
Marcel ARNOULD
Institut d’Astronomie et d’Astrophysique, ULB
and its implication on
A brief introduction
Nuclear decays and reactions via weak interaction play a key
role in many fields of stellar astrophysics
A larger variety of such processes can develop in stars than in
the laboratory
In addition
A large variety of Neutrino-Nucleus Interaction processes
including Neutral-Current processes
Temperature effects
:
Decay of thermally populated nuclear excited states
Temperature + density effects
:
Reduction of emitted lepton phase space (Pauli principle) at high
density + low temp. (Fermi-Dirac statistics)
Capture of e
+ 
, free  e
- 
:
Exo -, as well as endothermic transitions possible (Fermi energy)
Ionization
 :
Bound e
-
 rate = 
f
 (stellar conditions) (e.g. 
7
Be)
Bound state 
-
decay
Stellar plasma conditions affect 
-decay processes in
many ways
STARS = WORLD OF VARIABLE DECAY CONSTANTS !
Measurements
Back to Bound-State Beta-Decay
1947
1983-1987
1992
1996
1961
2005
Prediction
Daudel et al.
Bahcall
Takahashi
and Yokoi
Calculation
probabilities
163
Dy
Jung et al.
187
Re
Bosch et al.
205
Tl Bound/continuum
Oktsubo et al.
ESR: Experimental Storage
Ring  GSI Darmstadt
Remarkable Agreement !
An Obvious Pre-requisite :
vacancies in atomic shells (esp. lowest energy ones)
Population of ionized states in local thermodynamic
equilibrium : Saha equation
Population of given atomic state = 
f
(T, 
ρ
, mass ions,
ionization potentials, atomic partition function)
 Note complication:  atomic states of ion perturbed by :
Other bound electrons
Surrounding free electrons/ions
Ionisation potentials in stars smaller than
laboratory values
 (« Depression of continuum »)
Another important requirement:
The emitted electron must have a low enough energy to
efficiently populate a vacant atomic state
(Much work for atomic physicists !!)
Complications in the calculation
of energetics of transition
Q
n
 = Neutral atom ground state mass difference has to be
corrected
-
Differences between energies of initial and final atomic states
involved and total binding energies of electron clouds in
initial and final ions
-
Depression of continuum
(see Takahashi and Yokoi, Nucl. Phys. A404, 578, 1983 for details)
Complete ionization
Allowed transitions only
Comparison between bound-state beta-decay and
normal beta
-
-decay
The Bound-State Beta-Decay
and Nucleo-Cosmochronology
Evaluation of the age of Solar System nuclides T
nuc
 (time between beginning of
galactic nucleosynthesis in disc and present epoch ≈ 
 
«
 
age of Galaxy  »   T
G
)
Basis : use a suitable chronometric pair A (unstable) – B (stable/unstable)
Requirements for a good pair
I.
Decay half-life accurately known
II.
Half-life commensurable with galactic age
III.
Accurate abundance data in present Solar System (meteorites)
           A/B│
T
G
 (obs) (age of solar system known ~ 4.6 Gyr)
IV.
Good model for evolution of the nuclidic content of galactic disc up to
time of isolation of Solar System (a formidable problem !)
            A/B│
T
G
(th)
A/B│
T
G
 (obs)          A/B│
T
G
 (th)
  T
G
Most famed chronometric pairs for evaluation of T
G
232
Th (1.4 10
10 
y
)/
238
U (4.5 10
9
 
y
)
235
U (7 10
8 
y
)/
238
U (4.5 10
9
 
y
)
Poor predictive power !
(Yokoi et al., Astron. Astrophys.  117 (1983) 65)
187
Re (4.4 10
10 
y
)/
187
Os (stable)
(Reasonable) Hope !
Most famed chronometric pairs for evaluation of T
G
The 
187
 Re
-
 
187
Os Pair
ADVANTAGES
Apart from radiogenic (
187
Os)
RAD
 contribution from 
187
Re decay, 
187
Os made in
s-process
(
187
Os)
RAD 
= (
187
Os)
Θ
- (
187
Os)
s
Some problems, but …
INCONVENIENTS
187
Re clock runs differently in different stellar zones, interstellar medium
!Bound state Beta decay!
187
Os (EC) 
187
Re in certain stellar zones
Difficulties in predicting yields from individual stars
Difficulties in predicting galactic 
187
Re content at given time 0< t ≤ T
G
 
Beta-Decays in stellar plasmas and ionization
 The case of 
187
Re
5/2
+
~5X10
10
 
y
r
187
Re
75
-
187
Os
76
2.66 keV
   ½
-
134 keV
3/2
-
9.75 keV
 
Bound-state Beta-Decays in centrally H-burning stars
And now, the ultimate step !
… Put all the necessary ingredients [geochemical data,
astronomical observations, astrophysical modellings, nuclear,
atomic experiments and theory] into the grand galactic
blender
What comes out from the Re-Os recipe :
13  <  T
G  
<  18 G
y
r
(Latest news from Takahashi, Nucl. Phys. A718 (2003) 325c)
Not incompatible with other chronometric predictions
Clearly still a long way to go to improve predictions
~
~
Michel …..
!!! Your help would be greatly appreciated  !!!
You will have plenty of free time soon … to
become an astrophysicist at last
Illustration impact of bound-state beta-decay on
nucleosynthesis : the case of the production of 
164
Er
Production of the nuclides heavier than iron : the s-, r- and p-
processes
164
Er (Z=68, N=96) : An s- or/and p- process origin ?
All p-process models largely underproduce 
164
Er
s-process models cannot produce 
164
Er, … except if bound-
state 
-decay is invoked !
CONC. 1
 
94
96
98
162
164
166
160
162
164
Er 
68
Ho 
67
Dy 
66
« Normal » s-Process path
s- process path with 
163
Dy Bound-State Beta-Decay
e
-
+
-
St
(n,
)
-
e
-
Details of the s-process path 
164
Er
CONC. 2
The Bound State Beta-Decay of 
163
D
y
9/2
-
   167.34
9/2-     100.0
7/2
-
     73.44
7/2-     
4750
y
5/2
-
     163
D
y
                                     
163
 Ho
2.6 keV
Bound-State
Beta-Decay from
excited states
Continuum
electron
captures from
excited states
Takahashi and Yokoi
(1983)
With Bound-State Beta-
Decay, the s-process
could account for the
solar 
164
Er content
CONC. 3
S-Process production of 
186
Os, 
187
Os
186
Os
187
Os
185
Re
186
Re
187
Re
184
W
185
W
186
W
187
W
Z
N
76
75
74
110
111
112
113
ϐ
-
(n,
)
e
-
c
Ground-state (n,
) cross sections known experimentally … but complication due
to contribution to (n,
) rates of populated nuclear excited states (esp. 9.75 keV
first excited state of 
187
Os)
(some recent experimental and theoretical results, but some uncertainties
remain)
CONC. 4
The galactic blender
CONC. 5
Slide Note
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Nuclear decays and reactions, driven by weak interactions, are vital in stellar astrophysics. Various processes like bound-state beta-decay impact nucleosynthesis and cosmochronology. Specific processes in stars involve capture reactions, electron capture, and neutrino-nucleus interactions. Stellar plasma conditions influence decay processes significantly. Studies from 1983 to 2005 showcased the measurement and prediction accuracy in bound-state beta-decay. Understanding atomic vacancies and ionized states is crucial for explaining nuclear processes in stars.

  • Nuclear Decays
  • Stellar Astrophysics
  • Weak Interactions
  • Bound-State Beta-Decay
  • Nucleosynthesis

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  1. When Michels favorite tiny electrons fool the big atomic nuclei in the skies Marcel ARNOULD Institut d Astronomie et d Astrophysique, ULB By way of an illustration : the phenomenon of Bound-State Beta-Decay and its implication on Stellar Nucleosynthesis and Cosmochronology

  2. A brief introduction Nuclear decays and reactions via weak interaction play a key role in many fields of stellar astrophysics A larger variety of such processes can develop in stars than in the laboratory Common processes in normal lab conditions ???? : (Z,N) --> (Z+1, N 1) + ? + n? ????+: (Z,N) --> (Z-1, N+1) + ?+ + n? _ --> (Z-1, N+1) + n? Bound Electron Capture : (Z,N)+ eb

  3. Specific Processes in Stars _ --> (Z-1, N+1) + n? ????????? ? capture : (Z,N) + ec Positron Capture : (Z,N) + e+ --> (Z+1, N-1) + n? Bound-State -Decay : (Z,N) --> (Z+1, N-1) + n? In addition A large variety of Neutrino-Nucleus Interaction processes including Neutral-Current processes

  4. Stellar plasma conditions affect -decay processes in many ways Temperature effects: Decay of thermally populated nuclear excited states Temperature + density effects: Reduction of emitted lepton phase space (Pauli principle) at high density + low temp. (Fermi-Dirac statistics) Capture of e+ , free e- : Exo -, as well as endothermic transitions possible (Fermi energy) Ionization : Bound e- rate = f (stellar conditions) (e.g. 7Be) Bound state -decay STARS = WORLD OF VARIABLE DECAY CONSTANTS !

  5. Back to Bound-State Beta-Decay 1983-1987 19921996 2005 1947 1961 Measurements Calculation probabilities Prediction Daudel et al. 205Tl Bound/continuum Oktsubo et al. 187Re Bosch et al. Takahashi and Yokoi Bahcall 163Dy Jung et al. ESR: Experimental Storage Ring GSI Darmstadt Remarkable Agreement !

  6. An Obvious Pre-requisite : vacancies in atomic shells (esp. lowest energy ones) Population of ionized states in local thermodynamic equilibrium : Saha equation Population of given atomic state = f(T, , mass ions, ionization potentials, atomic partition function) Note complication: atomic states of ion perturbed by : Other bound electrons Surrounding free electrons/ions

  7. Ionisation potentials in stars smaller than laboratory values ( Depression of continuum ) (Much work for atomic physicists !!) Another important requirement: The emitted electron must have a low enough energy to efficiently populate a vacant atomic state

  8. Complications in the calculation of energetics of transition Qn = Neutral atom ground state mass difference has to be corrected - Differences between energies of initial and final atomic states involved and total binding energies of electron clouds in initial and final ions - Depression of continuum (see Takahashi and Yokoi, Nucl. Phys. A404, 578, 1983 for details)

  9. Comparison between bound-state beta-decay and normal beta--decay Complete ionization Allowed transitions only

  10. The Bound-State Beta-Decay and Nucleo-Cosmochronology Evaluation of the age of Solar System nuclides Tnuc (time between beginning of galactic nucleosynthesis in disc and present epoch age of Galaxy TG) Basis : use a suitable chronometric pair A (unstable) B (stable/unstable) Requirements for a good pair I. Decay half-life accurately known II. Half-life commensurable with galactic age III. Accurate abundance data in present Solar System (meteorites) A/B TG (obs) (age of solar system known ~ 4.6 Gyr) IV. Good model for evolution of the nuclidic content of galactic disc up to time of isolation of Solar System (a formidable problem !) A/B TG(th) A/B TG (obs) A/B TG (th) TG

  11. Most famed chronometric pairs for evaluation of TG Most famed chronometric pairs for evaluation of TG 232Th (1.4 1010 y)/238U (4.5 109y) 235U (7 108 y)/238U (4.5 109y) Poor predictive power ! (Yokoi et al., Astron. Astrophys. 117 (1983) 65) 187Re (4.4 1010 y)/187Os (stable) (Reasonable) Hope !

  12. The 187 Re-187Os Pair ADVANTAGES Apart from radiogenic (187Os)RAD contribution from 187Re decay, 187Os made in s-process (187Os)RAD = (187Os) - (187Os)s Some problems, but INCONVENIENTS 187Re clock runs differently in different stellar zones, interstellar medium !Bound state Beta decay! 187Os (EC) 187Re in certain stellar zones Difficulties in predicting yields from individual stars Difficulties in predicting galactic 187Re content at given time 0< t TG

  13. Beta-Decays in stellar plasmas and ionization The case of 187Re 3/2- 134 keV 9.75 keV 5/2+ 187Re75+ 5/2+ ~5X1010 yr Q=63.22keV - 3/2 1/2 2.66 keV - 9.75 keV 187Re 75 187Os 76 187Os75+(K shell) t1/2[y] Number of electrons bound to 187Re

  14. Bound-state Beta-Decays in centrally H-burning stars

  15. And now, the ultimate step ! Put all the necessary ingredients [geochemical data, astronomical observations, astrophysical modellings, nuclear, atomic experiments and theory] into the grand galactic blender What comes out from the Re-Os recipe : 13 < TG < 18 Gyr ~ ~ (Latest news from Takahashi, Nucl. Phys. A718 (2003) 325c) Not incompatible with other chronometric predictions Clearly still a long way to go to improve predictions

  16. Michel .. !!! Your help would be greatly appreciated !!! You will have plenty of free time soon to become an astrophysicist at last

  17. Illustration impact of bound-state beta-decay on nucleosynthesis : the case of the production of 164Er Production of the nuclides heavier than iron : the s-, r- and p- processes 164Er (Z=68, N=96) : An s- or/and p- process origin ? All p-process models largely underproduce 164Er s-process models cannot produce 164Er, except if bound- state -decay is invoked !

  18. CONC. 1

  19. CONC. 2 Details of the s-process path 164Er 98 96 94 e- + Er 68 162 164 166 (n, ) - Ho 67 - Dy 66 164 160 162 St e- Normal s-Process path s- process path with 163Dy Bound-State Beta-Decay

  20. CONC. 3 The Bound State Beta-Decay of 163Dy 9/2- 167.34 9/2- 100.0 7/2- 73.44 7/2- 4750y 2.6 keV 5/2- 163Dy 163 Ho Bound-State Beta-Decay from excited states With Bound-State Beta- Decay, the s-process could account for the solar 164Er content Takahashi and Yokoi Continuum electron captures from excited states (1983)

  21. CONC. 4 S-Process production of 186Os, 187Os Z 186Os 187Os - 76 (n, ) 185Re 186Re 187Re 75 e-c 184W 185W 186W 187W 74 N 110 111 112 113 Ground-state (n, ) cross sections known experimentally but complication due to contribution to (n, ) rates of populated nuclear excited states (esp. 9.75 keV first excited state of 187Os) (some recent experimental and theoretical results, but some uncertainties remain)

  22. CONC. 5 The galactic blender

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