Progress Update on Nuclear Data Research at LLNL
Bret Beck
Dave Heinrichs
Soon Kim
Ed Lent
Caleb Mattoon
Catherine Percher
Lucas Snyder
Ching-Yen Wu
Alan Yamanaka
Presented (on-line) to the Nuclear Data Advisory Group on December 3, 2020
Outline
•
TPC
•
PPAC
•
TSL issues
•
Photon production from thermal neutron radiative capture in Cadmium
•
LLNL Pulsed Spheres
•
NCSP AM Benchmark Intercomparison
•
TEX Update
•
PDV
•
ND2022
New fission TPC
239
Pu(n,f)/
235
U(n,f) data
Shape looks good !! An additional absolute normalization measurement planned for 2021.
240
Pu Fission Parallel Plate Avalanche Counter
Fig. 1
The exploded view of the electroplating
cell. The target frame can be seen in green
with a seal O-ring shown in red.
Fig. 2
The
PPAC
fission chamber on the bench for a
vacuum test. Isobutane connection to the chamber is
through the Poly-Flow tubing attached to the top. PPAC
signals are transmitted through the 12 electric vacuum
feedthroughs shown in the front cover (right side of the
picture).
Current status
:
•
Roger Henderson has demonstrated successfully that the fragile Al foil can stand multiple cycles of attach and detach from the
electroplating cell without damaging the foil integrity. This cell is shown in Fig. 1
. We
expect
to begin the electroplating of
240
Pu on
the thin aluminum foil of 2.5
m in
Jan/Feb 2021 and be completed by June 2021.
•
All
procured parts, including the chamber, target frames, thin metal foils, and cables, have arrived. Mounting the metal foils to the
target frames has been completed and they are now ready for electroplating. Cable creation is in progress.
The PPAC fission
chamber has been successfully tested for vacuum integrity, shown in Fig. 2.
240
Pu Fission Parallel Plate Avalanche Counter
Fig. 3
Photo showing the wiring inside the PPAC chamber
(fabricated by Sean McLaughlin).
Processing Thermal Neutron Scattering Laws
Discrepancies due to different interpolation and extrapolation assumptions in processing codes
113
Cd(n,g) Major Lines
EGAF normalization error
113
Cd(n,g) Spectrum
Belgya data normalized to
113
Cd thermal (n,g) cross section of 19959.758 barns in ENDF/B-VIII.0.
Silene CAAS Benchmark
Cd lined
ALARM-TRAN-CH2-SHIELD-002
Silene CAAS Benchmark Results
LLNL Pulsed Spheres – CH
2
Simplified Detailed
Model Model
NCSP Benchmark Intercomparison Study
As part of this project, LLNL is increasing our suite of criticality benchmarks
to increase the overlap with MORET (IRSN), VALID (ORNL) and WHISPER
(LANL) results. To date, 3,045 high-precision COG results are available for
the following ICSBEP benchmarks using ENDF/B-VII.1, ENDF/B-VIII.0 and
JEFF-3.3 libraries:
These benchmarks have been provided to the LLNL ARDRA and MERCURY
groups to assist in expanding their benchmark suites.
Example: LLNL COG and MCNP Results for U-233
TEX-TSL
FY21
Experiments
Additional TEX Baselines
NCSP Proposal
16
TEX-Pu
Five variations on the baseline configurations, including tantalum diluent,
will be published as PU-MET-MIXED-003 in 2021
Experiments with thicker polyethylene and Lucite moderators to provide
more testing for NCSU TSLs planned for execution in 2021
Additional variants under design to investigate
240
Pu and address
Hanford/SRS tank farm validation needs
TEX-HEU
Baseline experiments with HEU Jemima plates and poly executed in 2020
and will be benchmarked in 2021, for publication in 2022
Low Temperature experiments at -40C (-40F) with HEU final design
underway, address transportation and unheated facility validation needs
with the UK’s NNL
6
Li and chlorine diluted experiment design underway, address validation
need from Y-12 (electrorefining) and LANL (solutions) and provide a test for
ORNL
35
Cl evaluation
PDV – Second try is a winner !!
G
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v
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I
V
S
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V
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ND2022 International Nuclear Data Conference:
July 24 – 29, 2022 in Sacramento, CA
Held at the (renovated) SAFE Credit Union Convention Center
– Near state capitol & downtown Sacramento
15 min. from Sacramento airport – 2 hours from OAK / SF / Tahoe
Room blocks reserved at Sheraton, Residence Inn & Best Western
hotels
Nuclear Data Advisory Group received an online report from Lawrence Livermore National Laboratory detailing progress on various projects, including thermal neutron scattering laws processing, fission data measurements, and PPAC fission chamber development for 240Pu. The report outlines successful testing and upcoming plans for fission normalization measurements and electroplating of 240Pu. Various images illustrate the work in progress, showcasing advancements in nuclear data research.
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Presentation Transcript
LLNL Report Presented (on-line) to the Nuclear Data Advisory Group on December 3, 2020 Bret Beck Dave Heinrichs Soon Kim Ed Lent Caleb Mattoon Catherine Percher Lucas Snyder Ching-Yen Wu Alan Yamanaka LLNL-PRES-817232 This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. Lawrence Livermore National Security, LLC
Outline TPC PPAC TSL issues Photon production from thermal neutron radiative capture in Cadmium LLNL Pulsed Spheres NCSP AM Benchmark Intercomparison TEX Update PDV ND2022 2 LLNL-PRES-817232
New fission TPC 239Pu(n,f)/235U(n,f) data Shape looks good !! An additional absolute normalization measurement planned for 2021. 3 LLNL-PRES-817232
240Pu Fission Parallel Plate Avalanche Counter Current status: Roger Henderson has demonstrated successfully that the fragile Al foil can stand multiple cycles of attach and detach from the electroplating cell without damaging the foil integrity. This cell is shown in Fig. 1. We expect to begin the electroplating of 240Pu on the thin aluminum foil of 2.5 m in Jan/Feb 2021 and be completed by June 2021. All procured parts, including the chamber, target frames, thin metal foils, and cables, have arrived. Mounting the metal foils to the target frames has been completed and they are now ready for electroplating. Cable creation is in progress. The PPAC fission chamber has been successfully tested for vacuum integrity, shown in Fig. 2. Fig. 2 The PPAC fission chamber on the bench for a vacuum test. Isobutane connection to the chamber is through the Poly-Flow tubing attached to the top. PPAC signals are transmitted through the 12 electric vacuum feedthroughs shown in the front cover (right side of the picture). Fig. 1 The exploded view of the electroplating cell. The target frame can be seen in green with a seal O-ring shown in red. 4 LLNL-PRES-817232
240Pu Fission Parallel Plate Avalanche Counter Fig. 3 Photo showing the wiring inside the PPAC chamber (fabricated by Sean McLaughlin). 5 LLNL-PRES-817232
Processing Thermal Neutron Scattering Laws Discrepancies due to different interpolation and extrapolation assumptions in processing codes 6 LLNL-PRES-817232
113Cd(n,g) Major Lines EGAF normalization error 7 LLNL-PRES-817232
113Cd(n,g) Spectrum Belgya data normalized to 113Cd thermal (n,g) cross section of 19959.758 barns in ENDF/B-VIII.0. 8 LLNL-PRES-817232
Silene CAAS Benchmark Cd lined ALARM-TRAN-CH2-SHIELD-002 9 LLNL-PRES-817232
Silene CAAS Benchmark Results 10 LLNL-PRES-817232
LLNL Pulsed Spheres CH2 Simplified Detailed Model Model 11 LLNL-PRES-817232
NCSP Benchmark Intercomparison Study As part of this project, LLNL is increasing our suite of criticality benchmarks to increase the overlap with MORET (IRSN), VALID (ORNL) and WHISPER (LANL) results. To date, 3,045 high-precision COG results are available for the following ICSBEP benchmarks using ENDF/B-VII.1, ENDF/B-VIII.0 and JEFF-3.3 libraries: These benchmarks have been provided to the LLNL ARDRA and MERCURY groups to assist in expanding their benchmark suites. 12 LLNL-PRES-817232
Example: LLNL COG and MCNP Results for U-233 13 LLNL-PRES-817232
PMM-002 Results- TEX Pu Baselines 14 LLNL-PRES-817232
PMM-002 Results and Additional Work TEX-TSL FY21 Experiments Additional TEX Baselines NCSP Proposal 15 LLNL-PRES-817232
Planned Work for TEX TEX-Pu Five variations on the baseline configurations, including tantalum diluent, will be published as PU-MET-MIXED-003 in 2021 Experiments with thicker polyethylene and Lucite moderators to provide more testing for NCSU TSLs planned for execution in 2021 Additional variants under design to investigate 240Pu and address Hanford/SRS tank farm validation needs TEX-HEU Baseline experiments with HEU Jemima plates and poly executed in 2020 and will be benchmarked in 2021, for publication in 2022 Low Temperature experiments at -40C (-40F) with HEU final design underway, address transportation and unheated facility validation needs with the UK s NNL 6Li and chlorine diluted experiment design underway, address validation need from Y-12 (electrorefining) and LANL (solutions) and provide a test for ORNL 35Cl evaluation 16 16 LLNL-PRES-817232
PDV Second try is a winner !! Godiva-IV Surface Velocity 17 LLNL-PRES-817232
ND2022 International Nuclear Data Conference: July 24 29, 2022 in Sacramento, CA Held at the (renovated) SAFE Credit Union Convention Center Near state capitol & downtown Sacramento 15 min. from Sacramento airport 2 hours from OAK / SF / Tahoe Room blocks reserved at Sheraton, Residence Inn & Best Western hotels 18 LLNL-PRES-817232
