LIEBE Molten Metal Target Design at CERN-ISOLDE

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2/25/2025
5
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 High Power Targetry Workshop
1
T. De Melo Mendonca, 
M. Delonca
, D. Houngbo, C. Maglioni, L. Popescu, P. Schuurmans, T. Stora
(May 21, 2014)
Outline
Introduction/context
Proposed design
Diffusion simulations
Numerical results
Heat Exchanger (HEX)
Beam impact
Conclusion & next steps
2/25/2025
5
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 High Power Targetry Workshop
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Introduction/context…
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 High Power Targetry Workshop
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Introduction/context (1)
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 High Power Targetry Workshop
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Collaboration started in May 2012 for the LIEBE (Liquid Eutectic Lead Bismuth
Loop Target) project:
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WP1 : Coordination
   
CERN
  
T. Stora
 
WP2 : Conceptual Design and simulations
 
SCK-CEN
  
P. Schuurmans
 
WP3 : Construction, assembly
  
CERN
  
M. Delonca
 
WP4 : Instrumentation
   
CERN
  
T. Mendonca
 
WP5 : Safety and Licensing
  
CEA
  
A. Marchix
 
WP6 : Target characterization and analysis
 
PSI
  
D. Schumann
 
WP7 : Radiochemistry
   
SINP
  
S. Lahiri
 
WP8 : Offline commissioning
  
IPUL
  
K. Kravalis
 
WP9 : Online operation
  
CERN
  
T. 
Mendonca
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Introduction/context (2)
ISOLDE: 
on-line isotope mass separator @ CERN
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Instantaneous power: 
≈ 1 GW
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1.4 GeV
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3e13 protons/pulse
Cycle: 1.2 s
3 kW average power
Introduction/context (3)
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 High Power Targetry Workshop
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Proposed design…
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Proposed design (1)
Proposed by EURISOL
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Proposed design (2)
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Proposed design - 
main part 
(3)
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 High Power Targetry Workshop
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≈ 650 mm
Proposed design – 
HEX 
(4)
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 High Power Targetry Workshop
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Proposed design – 
HEX 
(5)
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 High Power Targetry Workshop
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5 working temperatures defined in
step of 100 
º
C
5 inlets on each side
1 outlet on each side
For each working temperature
defined, 
only
 two inlets are used
.
200 
ºC
300 
ºC
400 
ºC
500 
ºC
600 
ºC
Diffusion simulations …
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Diffusion simulations (1)
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Static units
Diffusion: model from Fujioka et
al. (NIM 186 (1981) 409)
Courtesy T. Mendonca, CERN
Diffusion optimized for droplets
shape
Need a grid on the container to
create the shower
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Holes diameter: 0.1 mm,
Thickness plate: 0.5 mm
Material: SS304L
Diffusion simulations (2)
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Improvement of diffusion with temperature
177
Hg (T
1/2
= 130 ms) as reference:
 Increasing droplet radius will decrease
the released fraction
 Diffusion efficiency of 38% for 100 ms,
44% for 200 ms in the diffusion chamber
Maximum operating temperature limited by
vapor pressure of LBE
Diffusion
Courtesy T. Mendonca, CERN
Diffusion simulations (3)
Conclusions
Diffusion efficiency is improved with:
Droplet shape
Temperature
Falling time of the droplets (lower outlet velocity, longer falling
distance)
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5
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 High Power Targetry Workshop
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Numerical results…
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Numerical results – 
HEX
 
(1)
Need to keep the target at the desired working temperature for
temperature ranging from 200 
º
C till 600 
º
C
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Numerical results – 
HEX
 
(2)
Assessment of HEX behavior with CFX
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Numerical results – 
HEX
 
(3)
2/25/2025
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 High Power Targetry Workshop
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Summary of results:
Numerical results – 
HEX
 
(4)
2/25/2025
5
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 High Power Targetry Workshop
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Conclusions
Temperature and power extraction are in the proper range (values have been
checked over the full range of temperature, from 200 
º
C up to 600 
º
C)
Further analysis must be computed considering bad thermal contact between
the different parts
Prototype will validate the design
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Numerical results – 
Beam impact 
(1)
Assessment of beam impact with Fluka &
       Ansys Autodyn
Geometry considered
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Container: 
Container: 
Stainless Steel 304, solid part,
Lagrangian part
Liquid: 
Liquid: 
LBE, SPH elements
Use of 40 gauges along beam axis
Isolde beam parameters
Numerical results – 
Beam impact 
(2)
Material definition
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 High Power Targetry Workshop
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Courtesy E. Noah, Un Geneva
Numerical results – 
Beam impact 
(3)
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 High Power Targetry Workshop
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Shock waves deposit energy onto the weakest
point of the container (grid part).
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Numerical results – 
Beam impact 
(4)
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 High Power Targetry Workshop
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Cavitation in the liquid will induce splashing of the LBE
and projection of droplets with very high velocity in the
diffusion chamber.
Deformation scale: *9
Numerical results – 
Beam impact 
(5)
Conclusions & Outlook
The geometry needs an improvement to avoid resonant shock waves
Impact of beam onto the container should be further investigated:
Negligible impact expected
Need more detailed simulation to prove it
Simulation must be computed for longer time
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 High Power Targetry Workshop
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Conclusion & next steps…
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Conclusion & next steps
Preliminary design is available, under
optimization
Test of the Heat Exchanger foreseen
Optimization of the irradiation container under
beam impact on-going
Off-line tests scheduled in the near future
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 High Power Targetry Workshop
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Thank you for your attention!
2/25/2025
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 High Power Targetry Workshop
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Thanks to all the contributors…
V. Barozier
A. P. Bernardes
K. Kravalis
F. Loprete
S. Marzari
R. Nikoluskins
F. Pasdeloup
A. Polato
H. Znaidi
… (and many others…)
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Back up slides…
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 High Power Targetry Workshop
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Introduction/context (4)
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Introduction/context (5)
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RIB intensity
 [s
-1 
μ
A
-1
]
Cross section
 [cm
2
]
Proton beam
intensity
 [s
-1 
μ
A
-1
]
Target density
 [atom 
cm
-2
]
Diffusion+effusion
efficiency
Ionization
efficiency
Radioactive ion beam (RIB) intensity:
Diffusion/effusion simulations (3)
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 High Power Targetry Workshop
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Effusion: Monte Carlo
The effusion efficiency is dependent on the geometry of the
container/diffusion chamber, the sticking time, the mean free path
and number of collisions with droplets and surface of containment.
Thanks to T. Mendonca
Sticking times of ~10
-12
 s – negligible
effect in efficiency
Effusion release
efficiencies between
22% and 34% for
residence times in the
diffusion chamber
between 100-200 ms
Estimated release
efficiencies (diff+eff)
of 
~ 8% 
for 100 ms
and 
~ 15% 
for 200 ms.
Concept 5 - Results
Feeder Volume
Irradiation Volume
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1 kg of LBE in Feeder
Volume,
2 feeder grids of 2520
apertures
1-mm or 0.5-mm thick
feeder grids
2520 evacuation
apertures
1.5-m/s inlet velocity
~0.2-bar pressure drop
Stable uniform flow
between 500 K – 1500 K
Houngbo D.- 
LIEBE project, Computational Fluid Dynamics (CFD) analysis
.- Workshop on Radioactive Ion Beam Production and
High-Power Target Stations.- Mol, Belgium, 16-18 September 2013.- [Presentation]
Numerical results – 
HEX
 
(3)
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 High Power Targetry Workshop
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Pressure in water for case LBE @ 200 
º
C
Velocity in water and LBE
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Numerical results – 
HEX
 
(4)
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 High Power Targetry Workshop
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Summary of results:
200 
ºC
300 
ºC
400 
ºC
500 
ºC
600 
ºC
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This project focuses on designing a molten metal target based on a Pb-Bi loop at CERN-ISOLDE. The aim is to validate the conceptual design for the EURISOL direct target by developing a prototype for CERN-ISOLDE. The collaboration began in May 2012 with specific work packages assigned for coordination, design, simulations, construction, safety, radiochemistry, and operational aspects. The target involves high power capabilities for short-lived isotopes. The introduction explains the context, ISOLDE's specifications, and the proposed design elements.

  • LIEBE
  • Molten Metal
  • Target Design
  • CERN-ISOLDE
  • EURISOL

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  1. LIEBE: Design of a molten metal target based on a Pb-Bi loop at CERN-ISOLDE T. De Melo Mendonca, M. Delonca, D. Houngbo, C. Maglioni, L. Popescu, P. Schuurmans, T. Stora (May 21, 2014) 5th High Power Targetry Workshop 1 2/25/2025

  2. Outline Introduction/context Proposed design Diffusion simulations Numerical results Heat Exchanger (HEX) Beam impact Conclusion & next steps 5th High Power Targetry Workshop 2 2/25/2025

  3. Introduction/context 5th High Power Targetry Workshop 3 2/25/2025

  4. Introduction/context (1) Aim of LIEBE target: validation of conceptual design for the EURISOL direct target by developing a prototype for CERN-ISOLDE. Some keywords: high power target, short-lived isotopes, Collaboration started in May 2012 for the LIEBE (Liquid Eutectic Lead Bismuth Loop Target) project: WP definition WP holder Coordinator WP1 : Coordination WP2 : Conceptual Design and simulations WP3 : Construction, assembly WP4 : Instrumentation WP5 : Safety and Licensing WP6 : Target characterization and analysis WP7 : Radiochemistry WP8 : Offline commissioning WP9 : Online operation CERN SCK-CEN CERN CERN CEA PSI SINP IPUL CERN T. Stora P. Schuurmans M. Delonca T. Mendonca A. Marchix D. Schumann S. Lahiri K. Kravalis T. Mendonca 5th High Power Targetry Workshop 4 2/25/2025

  5. Introduction/context (2) ISOLDE: on-line isotope mass separator @ CERN Proton beam from PSB: 1.4 GeV 2 A 3e13 protons/pulse Cycle: 1.2 s 3 kW average power Instantaneous power: 1 GW 5th High Power Targetry Workshop 5 2/25/2025

  6. Introduction/context (3) 5th High Power Targetry Workshop 6 2/25/2025

  7. Proposed design 5th High Power Targetry Workshop 7 2/25/2025

  8. Proposed design (1) Proposed by EURISOL 5th High Power Targetry Workshop 8 2/25/2025

  9. Current front end + target Proposed design (2) Main loop Pump/motor Current target unit Diameter: 300 mm 5th High Power Targetry Workshop 9 2/25/2025

  10. Proposed design - main part (3) Filling tank Container * Beam 650 mm HEX Diffusion chamber Pump pipes + heating/isolating elements all along the loop * D. Houngbo, SCK-CEN 5th High Power Targetry Workshop 10 2/25/2025

  11. Proposed design HEX (4) HEX LBE Casserole in between water and LBE LBE circulation Water block 5th High Power Targetry Workshop 11 2/25/2025

  12. Proposed design HEX (5) 5 working temperatures defined in step of 100 C 5 inlets on each side 1 outlet on each side 400 C 600 C For each working temperature defined, only two inlets are used. 500 C 200 C 300 C 5th High Power Targetry Workshop 12 2/25/2025

  13. Diffusion simulations 5th High Power Targetry Workshop 13 2/25/2025

  14. Diffusion simulations (1) Diffusion: model from Fujioka et al. (NIM 186 (1981) 409) ? ? =2.? 1 ?2 ?=1 ??+ ???? ?2 With ??= ? ???????????? ????????? ???? = ? = ?????? ?? ??????? ????????? ??????????? ?? ??????? ?? ??? ?? ??? ??= ???? ???? ?? ??????? ? = ?2 ? Static units Diffusion optimized for droplets shape Need a grid on the container to create the shower 10 mm Holes diameter: 0.1 mm, Thickness plate: 0.5 mm Material: SS304L Courtesy T. Mendonca, CERN 5th High Power Targetry Workshop 14 2/25/2025

  15. Diffusion simulations (2) 177Hg (T1/2= 130 ms) as reference: Diffusion Improvement of diffusion with temperature Increasing droplet radius will decrease the released fraction Diffusion efficiency of 38% for 100 ms, 44% for 200 ms in the diffusion chamber Maximum operating temperature limited by vapor pressure of LBE Courtesy T. Mendonca, CERN 5th High Power Targetry Workshop 15 2/25/2025

  16. Diffusion simulations (3) Conclusions Diffusion efficiency is improved with: Droplet shape Temperature Falling time of the droplets (lower outlet velocity, longer falling distance) 5th High Power Targetry Workshop 16 2/25/2025

  17. Numerical results 5th High Power Targetry Workshop 17 2/25/2025

  18. Numerical results HEX(1) Need to keep the target at the desired working temperature for temperature ranging from 200 C till 600 C Power contributions: Pump power extraction + - Beam Pump Pump Radiation Radiation power extraction - HEX Beam 330 to 990 W Pump 2 200 W 5th High Power Targetry Workshop 18 2/25/2025

  19. Numerical results HEX(2) Assessment of HEX behavior with CFX Dimensioning of an HEX: P = H S ?????? ???= ?2 ?1 1 ??? ? = 1 1+1 ln ?2 ?1 2 Problem: The HEX must extract less power @ 600 C than @ 200 C BUT power extracted depend on the surface of exchange, the average heat exchange coefficient and the temperature of both fluids involved -> need of a variable HEX! Water LBE Flow rate (l/s) T inlet ( C) T outlet ( C) 0.22 27 < 90 0.23 Variable Variable 5th High Power Targetry Workshop 19 2/25/2025

  20. Numerical results HEX(3) Summary of results: Example @ 600 C T max water ( C) P extracted (W) 200 C 300 C 400 C 500 C 600 C 78 83 73 68 79 3 180 3 050 2 890 2 820 2 650 Tmax water = 79 C Tmax LBE = 597 C 5th High Power Targetry Workshop 20 2/25/2025

  21. Numerical results HEX(4) Conclusions Temperature and power extraction are in the proper range (values have been checked over the full range of temperature, from 200 C up to 600 C) Further analysis must be computed considering bad thermal contact between the different parts Prototype will validate the design Temperature controlled with heating elements installed all along the loop 5th High Power Targetry Workshop 21 2/25/2025

  22. Numerical results Beam impact (1) Assessment of beam impact with Fluka & Ansys Autodyn Geometry considered Isolde beam parameters Container: Stainless Steel 304, solid part, Lagrangian part Liquid: LBE, SPH elements Use of 40 gauges along beam axis 5th High Power Targetry Workshop 22 2/25/2025

  23. Numerical results Beam impact (2) Material definition Standard variables @ 600 C. , Cp, k ??= ?0+ ? ?? ? =1 2 1 + =? ?? ? ?? Shock EOS (Linear model) Gruneisen model Us = shock velocity, = Gruneisen coefficient, ??= particle velocity, C0 and S = fitting parameters Failure mechanism Hydrodynamic tensile limit 2 values considered: -150 kPa and -1.9 GPa (no value available for LBE) Courtesy E. Noah, Un Geneva 5th High Power Targetry Workshop 23 2/25/2025

  24. Numerical results Beam impact (3) Analysis for 50 s (1 pulse = 32.6 s) under hydrodynamic tensile limit Shock waves deposit energy onto the weakest point of the container (grid part). Stresses up to 350 MPa (Yield = 390 MPa) in less than 1 ms. 5th High Power Targetry Workshop 24 2/25/2025

  25. Numerical results Beam impact (4) Analysis for 50 s (1 pulse = 32.6 s) over hydrodynamic tensile limit Deformation scale: *9 Cavitation in the liquid will induce splashing of the LBE and projection of droplets with very high velocity in the diffusion chamber. 5th High Power Targetry Workshop 25 2/25/2025

  26. Numerical results Beam impact (5) Conclusions & Outlook The geometry needs an improvement to avoid resonant shock waves Impact of beam onto the container should be further investigated: Negligible impact expected Need more detailed simulation to prove it Simulation must be computed for longer time 5th High Power Targetry Workshop 26 2/25/2025

  27. Conclusion & next steps 5th High Power Targetry Workshop 27 2/25/2025

  28. Conclusion & next steps Preliminary optimization design is available, under Test of the Heat Exchanger foreseen Optimization of the irradiation container under beam impact on-going Off-line tests scheduled in the near future 5th High Power Targetry Workshop 28 2/25/2025

  29. Thank you for your attention! 5th High Power Targetry Workshop 29 2/25/2025

  30. Thanks to all the contributors V. Barozier A. P. Bernardes K. Kravalis F. Loprete S. Marzari R. Nikoluskins F. Pasdeloup A. Polato H. Znaidi (and many others ) 5th High Power Targetry Workshop 30 2/25/2025

  31. Back up slides 5th High Power Targetry Workshop 31 2/25/2025

  32. Introduction/context (4) Specificity of RIBs (Radioactive Ion Beam) production via the ISOL (Isotope separation on-line) technique:Isolde target unit Extraction electrode Effusion Diffusion Ion source Target Transfer line Plasma Extracted ion beam Leaks Primary beam Condensation Neutrals Decay loss Leaks Leaks Release loss Isotope production Condensation Sidebands Multiplycharged Decay loss Decay loss 5th High Power Targetry Workshop 32 2/25/2025

  33. Introduction/context (5) Specificity of RIBs (Radioactive Ion Beam) production via the ISOL (Isotope separation on-line) technique:Isolde target unit Radioactive ion beam (RIB) intensity: Transfer line Heated: decrease adsorption in effusion process Cooled: trap condensable isobaric contaminants Target density [atom cm-2] Diffusion+effusion efficiency RIB intensity [s-1 A-1] ( ) = diff I N I + arg RIB prod t et prim beam eff ion Cross section [cm2] Proton beam intensity [s-1 A-1] Ionization efficiency Target Heating Diffusion improves with temperature 5th High Power Targetry Workshop 33 2/25/2025

  34. Diffusion/effusion simulations (3) Effusion: Monte Carlo The effusion efficiency is dependent on the geometry of the container/diffusion chamber, the sticking time, the mean free path and number of collisions with droplets and surface of containment. Sticking times of ~10-12s negligible effect in efficiency Effusion efficiencies 22% and 34% for residence times in the diffusion between 100-200 ms release between chamber Estimated efficiencies of ~ 8% for 100 ms and ~ 15% for 200 ms. release (diff+eff) Thanks to T. Mendonca 5th High Power Targetry Workshop 34 2/25/2025

  35. Concept 5 - Results 1 kg of LBE in Feeder Volume, 2 feeder grids of 2520 apertures 1-mm or 0.5-mm thick feeder grids 2520 evacuation apertures 1.5-m/s inlet velocity ~0.2-bar pressure drop Stable uniform flow between 500 K 1500 K Static-Pressures (Pa) Velocity Vectors (m/s) Feeder Volume Irradiation Volume 35 Houngbo D.- LIEBE project, Computational Fluid Dynamics (CFD) analysis.- Workshop on Radioactive Ion Beam Production and High-Power Target Stations.- Mol, Belgium, 16-18 September 2013.- [Presentation]

  36. Numerical results HEX(3) Example @ 600 C Velocity in water and LBE Tmax water = 79 C Tmax LBE = 597 C Pressure in water for case LBE @ 200 C 5th High Power Targetry Workshop 36 2/25/2025

  37. Numerical results HEX(4) Summary of results: 3610 T max water ( C) P extracted (W) Power extracted (W) 3110 200 C 300 C 400 C 500 C 600 C 200 C 300 C 400 C 500 C 600 C 78 83 73 68 79 3 180 3 050 2 890 2 820 2 650 2610 2110 1610 200 250 300 350 400 450 500 550 600 Temperature LBE (Deg C) 5th High Power Targetry Workshop 37 2/25/2025

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